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High harmonic generation from aligned molecules-amplitude and polarization 

Authors: Y. Mairesse ab;  J. Levesque ac;  N. Dudovich ad;  P. B. Corkum ae; D. M. Villeneuve a
Affiliations:   a National Research Council of Canada, Ottawa, Ontario, Canada
b CELIA, Universiteacute Bordeaux I, France
c INRS-Eacutenergie et Mateacuteriaux, Queacutebec, Canada
d Department of Physics of Complex Systems, Weizmann Institute of Science, Israel
e University of Ottawa, Ottawa, Canada
DOI: 10.1080/09500340802175766
Publication Frequency: 21 issues per year
Published in: journal Journal of Modern Optics, Volume 55, Issue 16 September 2008 , pages 2591 - 2602
First Published: September 2008
Formats available: HTML (English) : PDF (English)
Previously published as: Optica Acta: International Journal of Optics (0030-3909) until 1987
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Abstract

While high harmonic generation from atoms is relatively well understood, the ability to align gas-phase molecules opens an opportunity to more deeply understand the underlying physics. Many assumptions, such as the single active electron approximation, neglect of the Coulomb potential, the strong field approximation, and the assumption of plane waves, are being challenged by new experimental observations. We study high harmonic emission from aligned molecules such as N2, O2 and CO2. We present experimental measurements of the amplitude of the emission as a function of molecular angle, as well as the polarization state.
Keywords: attosecond; high harmonic generation; molecular alignment
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